By Faye Porter
What could you provide for a day on your grandmother's kitchen?
Leaning over the countertop, you think as she additional the flour?just a bit at a time?to the bowl of her outdated, yellow Sunbeam stand mixer. To her, cooking can have been as moment nature as atmosphere the desk. To you, it appeared similar to magic?the manner she skillfully positioned issues jointly to create the mouthwatering nutrition and exclusive cakes you loved at her desk. most probably, it's her culinary delights that experience set the bar for every little thing you've eaten due to the fact that. And let's face it, her pan fried red meat chops and home-baked banana bread make an individual else's models faded compared. if you are wishing for only a little extra time on your grandmother's kitchen?complete along with her tales and the thoughts of the comforting favorites she lovingly made for you?you're certain to embody this social gathering of grandmother's cooking. She'd be proud!
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Extra info for At My Grandmother's Table: Heartwarming Stories and Cherished Recipes from the South
This revealed formation of the (Z,E,E)-polyene 43, corresponding to a selective E/Z double bond isomerisation. Further irradiation led to the gradual disappearance of the two polyenes 43 and 44, accompanied by formation of tridachiahydropyrone (9). 18 Construction of (E,E,E)-polyene 44. Reagents and conditions: a Pd(PPh3)4, aq. KOH, THF, 80 °C, 55 % O O O hν, MeOH, rt. 19 The biomimetic conversion of 44 into 43, 9 and 93 irradiation resulted in the formation of a new, unexpected, product. The structure of the new photoproduct, named phototridachiahydropyrone (93), was determined by spectroscopic analysis and X-ray crystallography.
19). This revealed formation of the (Z,E,E)-polyene 43, corresponding to a selective E/Z double bond isomerisation. Further irradiation led to the gradual disappearance of the two polyenes 43 and 44, accompanied by formation of tridachiahydropyrone (9). 18 Construction of (E,E,E)-polyene 44. Reagents and conditions: a Pd(PPh3)4, aq. KOH, THF, 80 °C, 55 % O O O hν, MeOH, rt. 19 The biomimetic conversion of 44 into 43, 9 and 93 irradiation resulted in the formation of a new, unexpected, product. The structure of the new photoproduct, named phototridachiahydropyrone (93), was determined by spectroscopic analysis and X-ray crystallography.
The formation of 93 can be explained as arising from a photochemical [1,3]-sigmatropic rearrangement of tridachiahydropyrone (9). Whilst phototridachiahydropyrone (93) has not been isolated from natural sources, it is reasonable to assume that it is a natural product yet to be discovered. A further biosynthetic hypothesis, namely that tridachiahydropyrones B (12) and C (13), isolated as an inseparable mixture in 2000 by Schmitz and co-workers , were derived from a photochemical [4 + 2] cycloaddition of tridachiahydropyrone (9) with singlet oxygen, was also explored .